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the interaction), and the Lewis acidity and electrophilicity will have decreased. By the same token, it is more di cult to reduce (add a electron) than a methyl cation. 3. Use simple orbital interaction diagrams to explain each of the following: (a) The bonding in (b) Bonazzola and co-workers (Bonazzola, L.; Michaut, J. P.; Roncin, J., Can. J. Chem., 1988, 66, 3050) have shown by ESR spectroscopy that the singly ionized thiirane cation radical, [thiirane] X , forms a 1 : 1 complex with thiirane itself. Suggest a structure for the complex. Note: Thiirane is thiacyclopropane

Build the first parts of the data warehouse in very small, very fast steps, and carefully listen to the end users comments at the end of each step of development. Be prepared to make adjustments quickly. If available, use prototyping and allow the feedback loop to function using observations gleaned from the prototype.

To avoid inadvertently plotting to a Windows system printer when you should be plotting to a plotter, you can hide the display of Windows system printers in the Plot and Page Setup dialog boxes. Because these printers won t appear on the list of plotters, you can t plot to them. To hide system printers, choose Tools Options and click the Plot and Publish tab. In the General Plot Options section of the dialog box, check Hide System Printers and click OK.

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X: is NR 1 R 2 The substituent is converted to a Z substituent via the low-lying s orbital, and the ring is deactivated toward further electrophilic attack The ortho and para channels lead to products The interaction diagram for an X:-substituted pentadienyl cation, substituted in the 1-, 2-, and 3-positions, as models of the transition states for the ortho, meta, and para channels, are too complex to draw simple conclusions The HOMO and LUMO of the three pentadienyl cations with an amino substituent are shown in Figure 113 Notice that the LUMO of each is suitable to activate the C H bond at the saturated site toward abstraction by the base Curiously, the meta cation has the lowest LUMO and should most readily eliminate the proton The stabilities of the transition states should be in the order of the Huckel p energies.

Hunt s objectives for color reproduction provide a good summary of the problems encountered in color reproduction and how they can be addressed using concepts of basic and advanced colorimetry. It is interesting to note that these objectives were originally published long before issues in deviceindependent color imaging were commonly discussed (Hunt 1970). A slight rearrangement and simpli cation of Hunt s objectives can be used to de ne ve levels of color reproduction that provide a framework for modern color imaging systems.

These are 6 8X762j j, 6 8X499j j, and 6 8X718j j, respectively Thus the ortho and para channels are favored over the meta channel, and the ortho route is slightly preferred over the para route Experimentally, para substitution products are often the major ones in spite of there being two ortho pathways The predominance of para products is usually attributed to steric e ects Electrophilic Attack on Z-Substituted Benzenes The Z-substituted benzene (benzaldehyde, Figure 112) is not activated toward electrophilic attack since the HOMO of benzene is scarcely a ected No preferred site for attack of the electrophile can be deduced from inspection of the HOMOs The interaction diagram for a Z-substituted pentadienyl cation, substituted in the 1-, 2-, and 3-positions, as models of the transition states for the ortho, meta, and para channels are too complex to draw simple conclusions.

The HOMO and LUMO of the three pentadienyl cations with a formyl substituent are shown in Figure 114 The stabilities of the transition states should be in the order of the Huckel p energies These are 6 9X204j j, 6 9X203j j, and 6 9X129j j, respectively Thus, by SHMO, the ortho and meta channels are favored over the para channel, with no distinction between the ortho and meta pathways Experimentally, meta substitution products are usually the major ones, contrary to the SHMO predictions Either the SHMO method fails in this case or the predominance of meta products may be attributed to steric e ects..

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